The class of generating functions for completely monotone sequences (moments of finite positive measures on $[0,1]$) has an elegant characterization as the class of Pick functions analytic and positive on $(-\infty,1)$. We establish this and another such characterization and develop a variety of consequences. In particular, we characterize generating functions for moments of convex and concave probability distribution functions on $[0,1]$, and we provide a simple analytic proof that for any real $p,r>0$, the Fuss-Catalan or Raney numbers $\frac{r}{pn+r}\binom{pn+r}{n}$, $n=0,1,\ldots$ are the moments of a probability distribution on some interval $[0,\tau]$ if and only if $p\ge1$ and $p\ge r$.

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We consider singular integral operators of the form (a)$Z$_{1}L^{−1}Z_{2}, (b)$Z$_{1}Z_{2}L^{−1}, and (c)$L$^{−1}Z_{1}Z_{2}, where$Z$_{1}and$Z$_{2}are nonzero right-invariant vector fields, and$L$is the$L$^{2}-closure of a canonical Laplacian. The operators (a) are shown to be bounded on$L$^{p}for all$p$∈(1, ∞) and of weak type (1, 1), whereas all of the operators in (b) and (c) are not of weak type ($p, p$) for any$p$∈[1, ∞).