It is well known that group is a set with an algebra operation, which is often denoted by G . A simple group is the group which has only the 2 trivial normal subgroups. The importance of the simple groups may analogue to the prime numbers in the number theory. The classification of the finite simple groups was the central problem of 20th century’s’ algebra. In this research report, we use Sylow theorem, Burnside theorem, group action and some other elementally group theory methods to obtain some criteria of simple group . By using these criteria we determine the possible simple groups whose order less than 700. Generalizes the results in the reference [1]，[2]， [3]，[4].We conclude that Theorem A group G of order less or equal than 700 could not be simple except for |G|∈{60,168,360,504,660 and all primes}.